期刊
ORGANIC LETTERS
卷 20, 期 14, 页码 4337-4340出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b01762
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资金
- CSC
- DFG [EXC 1069, SFB-TRR 88]
A facile insertion of ruthenium into aromatic C-H and allylic C-N bonds are the key steps in a [Ru(p-cymene)Cl-2](2)-catalyzed ortho-C-H allylation of benzoic acids. This protocol allows drawing on the large pool of allylic amines for state-of-the-art ortho-functionalizations of arenes, turning neutral amines into leaving groups. Concise syntheses of biologically active compounds provide further evidence of the synthetic potential of this methodology.
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