期刊
ORGANIC LETTERS
卷 20, 期 3, 页码 612-615出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b03735
关键词
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资金
- KAKENHI from JSPS [25713002, 17H03025, JP16H01043]
- MEXT
- Shorai Foundation For Science and Technology
- Grants-in-Aid for Scientific Research [16K18856] Funding Source: KAKEN
Waste-free catalytic assembly of alpha-amino acids is fueled by a multiboron catalyst that features a characteristic B3NO2 heterocycle, providing a versatile catalytic protocol wherein functionalized natural alpha-amino acid units are accommodated and commonly used protecting groups are tolerated. The facile dehydrative conditions eliminate the use of engineered peptide coupling reagents, exemplifying a greener catalytic alternative for peptide coupling. The catalysis is sufficiently robust to enable pentapeptide synthesis, constructing all four amide bond linkages in a catalytic fashion.
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