期刊
ORGANIC LETTERS
卷 20, 期 9, 页码 2787-2791出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b00745
关键词
-
资金
- Council of Scientific and Industrial Research (CSIR)
- INSA Senior Scientist award
- INSA, New Delhi
A Lewis acid catalyzed regioselective C-C bond is constructed through beta-addition of deconjugated butenolides with p-quinone methides in a 1,6-conjugate addition manner. Interestingly, Lewis acid catalyzed vinylogous Mukaiyama-Michael reaction of silyloxyfurans with p-QMs proceeds selectively through the alpha or gamma position exclusively. The reaction is mild with broad substrate scope, thus allowing easy access to a wide range of bis-arylated alpha-/beta-/gamma-substituted butenolides.
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