期刊
ORGANIC LETTERS
卷 20, 期 3, 页码 792-795出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b03934
关键词
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资金
- French National Research Agency (ANR) as part of the Investissements d'Avenir program [ANR-11-IDEX-0003-02, CHARMMMAT ANR-11-LABX-0039]
- French National Research Agency (ANR) (Labex SynOrg) [ANR-11-LABX-0029]
- Universite de Versailles Saint Quentin
- Centre National de la Recherche Scientifique (CNRS)
An efficient domino polycyclization combining different classes of pericyclic reactions leads to complex spiroxindoles under mild conditions. This domino process represents a rare example of an in situ formation of cyclopentadienol derivatives from an interrupted iso-Nazarov electrocyclization of 2,4-dienals and their use in [4 + 2] cycloaddition reactions. According to the reaction conditions, different polycyclic architectures are obtained in good yields and excellent diastereoselectivities.
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