期刊
ORGANIC LETTERS
卷 20, 期 10, 页码 3049-3052出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b01079
关键词
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资金
- National Natural Science Foundation of China [21772129, 21502124]
- Fok Ying Tung Education Foundation [161013]
- 973 Project from the MOST of China [2015CB856600]
- Sichuan Provincial Department of Education [17ZA0219]
- Neijiang Normal University [KF10076]
A selective oxy-alkylation of allylamines with unactivated alkyl bromides and CO2 via visible-light-driven palladium catalysis is reported. The commercially available Pd(PPh3)(4) is used as the sole catalyst in this three component reaction. A variety of tertiary, secondary, and primary alkyl bromides undergo reactions to generate important 2-oxazolidinones in high yields and selectivity. The mild reaction conditions, easy scalability, and facile derivatization of products provide great potential for application in organic synthesis and pharmaceutical chemistry.
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