期刊
ORGANIC ELECTRONICS
卷 62, 期 -, 页码 548-553出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.orgel.2018.06.029
关键词
N-type organic thin-film transistors; Branched alkyl chain; Solution process; High electron mobility; Thermal durability
资金
- JSPS KAKENHI [15H02196, 16K05900]
- Strategic Promotion of Innovative Research and Development from JST
Single-crystal organic thin-film field-effect transistors (OTFTs) have been actively studied because they are regarded as an ideal platform for charge carrier transport phenomena in small-molecule organic materials. Moreover, recently developed solution-based techniques to grow single-crystalline thin films have attracted industrial attention beyond fundamental physics. In this work, one of the solution-based techniques, namely, the edgecasting method, was employed to study single-crystal OTFTs of n-type organic semiconductors, dimerized naphtho[2,3-b]thiophene diimides, with linear and branched alkyl chains. A high electron mobility of >1 cm(2)V(-1)s(-1) and an excellent thermal durability were observed in the branched alkyl-chain derivative, while the OTFT based on linear alkyl-substituted one showed clear degradation of mobility after thermal annealing. Therefore, this work will demonstrate a potential availability of branched alkyl chains for improving carrier mobility and thermal durability with large-scalable printing methods.
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