4.8 Article

Large magneto-optical Kerr effect and imaging of magnetic octupole domains in an antiferromagnetic metal

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NATURE PHOTONICS
卷 12, 期 2, 页码 73-+

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NATURE PUBLISHING GROUP
DOI: 10.1038/s41566-017-0086-z

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资金

  1. CREST [JPMJCR15Q5]
  2. Japan Science and Technology Agency from Ministry of Education, Culture, Sports, Science, and Technology of Japan [15H05882, 15H05883]
  3. Japanese Society for the Promotion of Science (JSPS) [R2604, 16H02209]
  4. US Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division within the Spin Physics programme [DEAC02-05CH11231, KC2206]
  5. Gordon and Betty Moore Foundation's EPiQS Initiative at UC Berkeley [GBMF4537]
  6. SHINES, an Energy Frontier Research Center of the US Department of Energy [SC0012670]
  7. QuantEmX grant from ICAM
  8. Gordon and Betty Moore Foundation [GBMF5305]
  9. US Department of Energy, office of Basic Energy Sciences, Division of Material Sciences and Engineering [DE-FG02-08ER46544]
  10. [DE-SC0009390]
  11. Grants-in-Aid for Scientific Research [15K17713, 16H02209, 15H05882] Funding Source: KAKEN

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The magneto-optical Kerr effect (MOKE) has been intensively studied in a variety of ferro-and ferrimagnetic materials as a powerful probe for electronic and magnetic properties(1-3) and for magneto-optical technologies(4). The MOKE can be additionally useful for the investigation of the antiferromagnetic (AF) state, although thus far limited to insulators(5-9). Here, we report the first observation of the MOKE in an AF metal. In particular, we find that the non-collinear AF metal Mn3Sn (ref. 10) exhibits a large zero-field Kerr rotation angle of 20 mdeg at room temperature, comparable to ferromagnetic metals. Our first-principles calculations clarify that ferroic ordering of magnetic octupoles(11) produces a large MOKE even in its fully compensated AF state. This large MOKE further allows imaging of the magnetic octupole domains and their reversal. The observation of a large MOKE in an AF metal will open new avenues for the study of domain dynamics as well as spintronics using antiferromagnets(12-16)

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