4.8 Article

Ultrafast Graphene Light Emitters

期刊

NANO LETTERS
卷 18, 期 2, 页码 934-940

出版社

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.7b04324

关键词

Graphene; ultrafast light emitter; thermal radiation; van der Waals heterostructure; optoelectronics

资金

  1. Columbia University SEAS Translational Fellow program
  2. Office of Naval Research [N00014-13-1-0662]
  3. DOE-BES grant [DE-FG02-00ER45799]
  4. Center for Excitonics, an Energy Frontier Research Center - U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0001088]
  5. National Research Foundation of Korea - Korea government [NRF-2015R1A2A1A10056103, SRC2016R1A5A1008184]
  6. NRF grant - Korea government [2017R1A2B3011586]
  7. third Stage of Brain Korea 21 Plus Project
  8. DARPA grant [FA8650-16-2-7640]
  9. Elemental Strategy Initiative
  10. JSPS KAKENHI, grant [JP15K21722]
  11. National Science Foundation [DMR-1411107]
  12. Air Force Office of Scientific Research [FA9550-12-1-0119]

向作者/读者索取更多资源

Ultrafast electrically driven nanoscale light sources are critical components in nanophotonics. Compound semiconductor-based light sources for the nanophotonic platforms have been extensively investigated over the past decades. However, monolithic ultrafast light sources with a small footprint remain a challenge. Here, we demonstrate electrically driven ultrafast graphene light emitters that achieve light pulse generation with up to 10 GHz bandwidth across a broad spectral range from the visible to the near-infrared. The fast response results from ultrafast charge-carrier dynamics in graphene and weak electron-acoustic phonon-mediated coupling between the electronic and, lattice degrees of freedom. We also find that encapsulating graphene with hexagonal boron nitride (hBN) layers strongly modifies the emission spectrum by changing the local optical density of states, thus providing up to 460% enhancement compared to the gray-body thermal radiation for a broad peak centered at 720 run. Furthermore, the hBN encapsulation layers permit stable and bright visible thermal radiation with electronic temperatures up to 2000 K under ambient conditions as well as efficient ultrafast electronic cooling via near-field coupling to hybrid polaritonic modes under electrical excitation. These high-speed graphene light emitters provide a promising path for on-chip light sources for optical communications and other optoelectronic applications.

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