期刊
NANO LETTERS
卷 18, 期 2, 页码 1259-1263出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.7b04855
关键词
Biomembranes; vesicles; Janus particles; particle adsorption; bending energy; membrane-mediated interactions
类别
资金
- Deutsche Forschungsgemeinschaft (DFG) [1524]
Besides direct particle particle interactions, nanoparticles adsorbed to biomembranes experience indirect interactions that are mediated by the membrane curvature arising from particle adsorption.. In this Letter, we show that the curvature-mediated interactions of adsorbed Janus particles depend on the initial curvature of the membrane prior to adsorption, that is, on whether the membrane initially bulges toward or away from the particles in our simulations. The curvature-mediated interaction Can be strongly attractive for Janus particles adsorbed to the outside of a membrane vesicle, which initially bulges away from the particles. For Janus particles adsorbed to the vesicle inside, in contrast, the curvature-mediated interactions are repulsive. We find that the area fraction of the adhesive Janus particle surface is an important control parameter for the curvature-mediated interaction and assembly of the particle, besides the initial membrane curvature.
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