期刊
ULTRAFAST IMAGING AND SPECTROSCOPY
卷 8845, 期 -, 页码 -出版社
SPIE-INT SOC OPTICAL ENGINEERING
DOI: 10.1117/12.2023391
关键词
molecular imaging; laser alignment; ultrafast electron diffraction; structural reconstruction
Three-dimensional imaging of molecules in the gas phase has been an important but challenging task, since the randomly oriented molecules only provide one-dimensional structural information. In this work, we show that a three-dimensional structure can be reconstructed from ultrafast electron diffraction from impulsively laser-aligned molecules. The diffraction pattern is taken at the maximum degree of alignment, around two picoseconds after the excitation of the laser. An iterative retrieval algorithm is developed to resolve the problem generated by imperfect alignment and a holographic algorithm is used to reconstruct molecular structure.
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