期刊
MACROMOLECULAR RAPID COMMUNICATIONS
卷 39, 期 14, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/marc.201700715
关键词
all-polymer solar cells (all-PSC); naphthalene diimide (NDI); non-fullerene acceptors; PTB7-Th; thianaphthene-fused perylenediimde (TDI)
资金
- National Key Research and Development Program of China [2017YFA0206600]
- Key Research Program of Frontier Sciences, Chinese Academy of Sciences [QYZDB-SSW-SLH033]
- National Natural Science Foundation of China (NSFC) [51473040, 51673048, 21602040, 21504019, 51773046]
- National Natural Science Foundation of Beijing [2162045]
A novel n-type polymer of PTDI-T based on asymmetric rylene diimide and thiophene is designed and synthesized. The highest power conversion efficiency of 4.70% is achieved for PTB7-Th: PTDI-T-based devices, which is obviously higher than those of the analogue polymers of PPDI-2T and PDTCDI. When using PBDB-T as a donor, an open-circuit voltage (V-OC) as high as 1.03 V is obtained. The results indicate asymmetric rylene diimide is a kind of promising building block to construct n-type photovoltaic polymers.
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