期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 140, 期 10, 页码 3555-3559出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.8b01005
关键词
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资金
- NSFC [21372268, 21772017]
- Fundamental Research Funds for the Central Universities [106112016-CDJZR228806]
1,2-Benzdiyne equivalents possess the unique property that they can react with two arynophiles through iteratively generated 1,2- and 2,3-aryne intermediates. Upon rational modification on the second leaving group of these aryne precursors, a domino aryne annulation approach was developed through a nucleophilic-ene reaction sequence. Various benzo-fused N-heterocyclic frameworks were achievable under transition metal-free conditions with a broad substrate scope.
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