期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 140, 期 4, 页码 1243-1246出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.7b12864
关键词
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资金
- MIT
- JGP, Kyoto University
- NSF graduate fellowship (NSF-GRFP)
This report details a new method for site-selective methylene oxidation adjacent to azaheterocydes. A dual catalysis approach, utilizing both an iron Lewis acid and an organic hydroxylamine catalyst, proved highly effective. We demonstrate that this method provides complementary selectivity to other known catalytic approaches and represents an improvement over current heterocycle-selective reactions that rely on stoichiometric activation.
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