期刊
JOURNAL OF SUPERCRITICAL FLUIDS
卷 134, 期 -, 页码 197-203出版社
ELSEVIER
DOI: 10.1016/j.supflu.2017.12.004
关键词
Metal-organic framework; Porous coordination polymer; Covalent organic framework; Supercritical fluid; Drying; Impregnation
资金
- JSPS KAKENHI [16K06850]
- Yoshida Science and Technology Foundation
- Matching Planer Program from the Japan Science and Technology Agency (JST) [MP28116808247]
- Grants-in-Aid for Scientific Research [16K06850] Funding Source: KAKEN
The synthesis and processing of porous materials is a particularly fertile area for supercritical fluid (SCF) technology. Well-designed metal-organic hybrid porous materials such as metal-organic frameworks (MOFs) and porous coordination polymers (PCPs), which are constructed from metal-containing nodes and organic linkers, have recently been recognized as an intriguing class of crystalline nanoporous materials with a wide variety of potential applications in areas including gas storage, compound separation, biomedicine, chemical sensing, and catalysis. Furthermore, covalent organic frameworks (COFs) constructed from light elements have been developed. Recent research in the rapidly expanding field of MOFs, PCPs and COFs has demonstrated that SCF technologies, such as drying, impregnation, and synthesis, are effective approaches for processing and improving MOFs, PCPs and COFs. This short review describes the processing of MOFs, PCPs and COFs using supercritical CO2 and its mixtures. Selected examples are presented, and current achievements and challenges are summarized.
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