期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 83, 期 15, 页码 8331-8340出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.8b01026
关键词
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资金
- Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP, Sao Paulo, Brazil) [FAPESP 2017/18400-6]
- Faepex-UNICAMP [FAPESP 2017/18400-6]
A visible-light-driven strategy for hydroacylation and epoxyacylation of olefins in water using methylene blue as photoredox catalyst and persulfate as oxidant is reported. In this unprecedented unified approach, two different transformations are accomplished using only one set of reagents. The method has a broad scope spanning a range of aromatic and aliphatic aldehydes as well as conjugated and nonconjugated olefins to deliver ketones and epoxyketones from abundant and inexpensive chemical feedstocks.
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