期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 83, 期 12, 页码 6477-6488出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.8b00758
关键词
-
资金
- NSFC [21525208, 21472186]
- Dalian Institute of Chemical Physics (Chinese Academy of Sciences)
Redox-neutral synthesis of isoquinolinium salts via C-H activation of presynthesized or in situ formed imines and coupling with alpha-diazo ketoesters has been realized, where a zinc salt promotes cyclization as well as provides a counteranion. Under three-component conditions, both ketone and aldehydes are viable arene sources. The coupling of imines with diazo malonates under similar conditions afforded isoquinolin-3-ones as the coupling product.
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