期刊
JOURNAL OF CHEMICAL PHYSICS
卷 148, 期 2, 页码 -出版社
AMER INST PHYSICS
DOI: 10.1063/1.5006947
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资金
- CAPES
- CNPq
- INCT-FCx
- US-AFOSR [FA9550-16-1-0280]
- PNDP-Capes Project [PNPD20132533]
In the present work, we investigate a gas-liquid transition in a two-component Gaussian core model, where particles of the same species repel and those of different species attract. Unlike a similar transition in a one-component system with particles having attractive interactions at long separations and repulsive interactions at short separations, a transition in the two-component system is not driven solely by interactions but by a specific feature of the interactions, the correlations. This leads to extremely low critical temperature, as correlations are dominant in the strong-coupling limit. By carrying out various approximations based on standard liquid-state methods, we show that a gas-liquid transition of the two-component system poses a challenging theoretical problem. Published by AIP Publishing.
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