期刊
JOURNAL OF ALLOYS AND COMPOUNDS
卷 740, 期 -, 页码 1159-1164出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.jallcom.2018.01.080
关键词
CaCu3Ti4O12 ceramics; Dielectric loss; IBLC; Insulating barrier layer; TiO2
资金
- National Natural Science Foundation of China [51602214, 11404236, 11604234]
- Natural Science Foundation of Shanxi Province [2015021026, 201601D202010]
- China Scholarship Council [2016081409162]
The large low-frequency dielectric loss of CaCu3Ti4O12 (CCTO) ceramics limit their applications. According to the internal barrier layer capacitance effect, which is the most widely accepted explanation for the giant-epsilon' phenomenon of CCTO ceramics, increasing the resistance of grain boundary is an effective way to reduce their low-frequency dielectric loss. In this work, CCTO/TiO2 composite ceramics with coreshell structure were prepared by sol-gel-like method, and their crystalline structures, microstructures, dielectrical properties and complex impedance were investigated systematically. The results show that the room temperature low-frequency dielectric loss of our CCTO-based ceramics decreased significantly by TiO2-doping and annealing in oxygen, which should be attributed to the increasing resistance of the insulating grain boundary. (C) 2018 Elsevier B.V. All rights reserved.
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