4.7 Article

Influences of the perforation on effective transport properties of gas diffusion layers

期刊

出版社

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ijheatmasstransfer.2018.05.016

关键词

Gas diffusion layer; Effective transport property; Perforation; Lattice Boltzmann method; Saturation; Multiple-relaxation-time

资金

  1. 13-5 National Key Research Project of China [2017YFB0102702]
  2. Key Project of International Joint Research of National Natural Science Foundation of China [51320105004]
  3. LANL's LDRD Program

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In this paper, the through-plane and in-plane effective transport properties, including permeability, diffusivity and thermal conductivity, of the perforated gas diffusion layer (GDL) are predicted using multiple-relaxation-time (MRT) lattice Boltzmann method (LBM) based on stochastic reconstructed microstructures. When predicting effective thermal conductivities of GDL, the effect of anisotropic conductive property of fibers is considered. The effective transport properties of dry perforated GDL are fitted as a function of perforation diameter and porosity. It is found that the permeability and effective diffusivity of GDL increase with perforation diameter and porosity while the effective thermal conductivity decreases. The two-phase LBM is adopted to simulate water distributions in perforated GDLs, and dependences of effective transport properties on saturation are then obtained. The results show that: the existence of the perforation significantly affects the water transport in hydrophobic perforated GDLs if its diameter is larger than the average pore size of GDL. The effective permeability and diffusivity of GDL decrease while effective thermal conductivity increases with saturation. The effective transport properties of perforated GDLs change less significantly with saturation than those of non-perforated GDL if the water droplet intruding into the perforation is displaced, while change more rapidly with saturation if the water droplet remains inside the perforation. (C) 2018 Published by Elsevier Ltd.

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