期刊
INORGANIC CHEMISTRY
卷 57, 期 15, 页码 9251-9259出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.inorgchem.8b01271
关键词
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资金
- National Natural Science Foundation of China (NSFC) [51672265, 51672266, 21521092, 51750110511, 51672257, 51672259]
- Key Research Program of Frontier Sciences, CAS [YZDY-SSW-JSC018]
- National Basic Research Program of China [2014CB643803]
- Scientific and Technological Department of Jilin Province [20150520029JH, 20170414003GH]
- Jiangmen Innovative Research Team Program [[2017]385]
- Major program of basic research and applied research of Guangdong Province [2017KZDXM083]
- Distinguished Scientist Fellowship Program of King Saud University
- Deanship of Scientific Research at King Saud University [RG-1939-038]
In the pursuit of high-quality W-LED lighting, the precise control of emission color of phosphor materials is indispensable. Herein we report a series of single-composition Bi3+-doped LiCa3MgV3O12 garnet-structure phosphors, whose emission colors under n-UV excitation could be tuned from bluish green (480 nm) to yellow (562 nm) on the basis of local lattice distortion and VO43- -> Bi3+ energy transfer. Furthermore, full-color luminescence tuning from bluish green to orangish red across the warm white light region was successfully achieved by designing VO43- -> Bi3+ -> Eu3+ energy transfers. More interestingly, the thermal stabilities of as-prepared samples were gradually enhanced through designing VO43-/Bi3+ -> Eu3+ energy transfers. This work provides a new perspective for color tuning originating from simultaneous local lattice distortion and multiple energy transfers.
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