期刊
INORGANIC CHEMISTRY
卷 57, 期 8, 页码 4230-4233出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.inorgchem.8b00106
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资金
- NSFC [21302072, 11722433, 21776119]
- PAPD
- TAPP of Jiangsu Higher Education Institutions
A photoactive triazolobenzothiadiazole (TBTD)-conjugated terphenyldicarboxylate (TPDC) linker was introduced into a porous and robust UiO-68 isoreticular zirconium metal-organic framework (denoted as UiO-68-TBTD) by the de novo synthetic approach of mixed TPDC struts. Under blue-light-emitting-diode irradiation, UiO-68-TBTD can serve as a heterogeneous photocatalyst for the highly efficient and selective oxidation of a sulfur mustard simulant (2-chloroethyl ethyl sulfide) to the corresponding much less toxic sulfoxide product, with a half-life of only 3 min in the open air atmosphere.
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