期刊
GREEN CHEMISTRY
卷 20, 期 14, 页码 3203-3209出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8gc01211c
关键词
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资金
- French National Research Agency [ANR-15-CE07-0018-01]
- Chevreul Institute [FR 2638]
- Ministere de l'Enseignement Superieur, de la Recherche et de l'Innovation
- Region Hauts-de-France
- FEDER
- Agence Nationale de la Recherche (ANR) [ANR-15-CE07-0018] Funding Source: Agence Nationale de la Recherche (ANR)
High performances in the conversion of ethanol to 1,3-butadiene were achieved with a Zn(ii) and Ta(v) catalyst supported on TUD-1, a mesoporous silica. The selectivity reached 73% after 3 h at 94% conversion. At an increased ethanol flow, the initial productivity increased to 2.45 g(1,3-BD) g(cat)(-1) h(-1), which remained stable for 60 h on stream, making it the most productive catalyst according to the literature. Preliminary characterization suggests that its morphological and acid properties contribute to these exceptional performances.
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