期刊
FUEL PROCESSING TECHNOLOGY
卷 176, 期 -, 页码 101-106出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.fuproc.2018.03.016
关键词
Carbon dioxide; Carbon monoxide; Fischer-Tropsch reaction; Nanoparticles; Cobalt; Metal-organic framework MIL-53(Al); DRIFTS; PXRD
资金
- Ministry of Education and Science of the Russian Federation [K2-2017-011]
- Russian Science Foundation [14-50-00126]
A novel 10%Co/MIL-53(Al) nanohybrid based on the microporous metal-organic framework MIL-53(Al) prepared by MW-assisted synthesis exhibits the properties of a bifunctional catalyst with activity in CO2 hydrogenation to CO and consecutive synthesis of liquid hydrocarbons from carbon monoxide formed. The observed increase in the CO2 conversion in comparison with the thermodynamically possible conversion is assumed to be due to the expected shift of the equilibrium toward the formation of CO as a result of its further rapid conversion to hydrocarbons by the Fisher-Tropsch reaction.
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