期刊
FUEL PROCESSING TECHNOLOGY
卷 133, 期 -, 页码 220-226出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.fuproc.2015.02.004
关键词
NH3-SCR; Fe/beta; Ce doping; Hydrothermal aging; SO2 resistance
资金
- Nature Science Foundation of China [21177110]
- Zhejiang Leading Team of Science and Technology Innovation [2009R50020]
The Ce doping Fe/beta catalysts were prepared by an easy incipient wetness impregnation method and characterized using various analytical techniques, including H-2-TPR, XRD, UV-vis and XPS. The results demonstrated that the addition of cerium effectively improved the deNO performance, hydrothermal stability and 503 resistance of the Fe/beta catalyst for the selective catalytic reduction (SCR) of NOx by NH3. The finely dispersed iron oxide nanoparticles on the surface of Ce-Fe/beta catalysts and the compensative effect of cerium are dominating reasons for high catalytic performance. The Ce doping enhanced the hydrothermal stability of the Fe/beta catalyst because it could control the growth of iron oxides and stabilize the dispersed iron species. Suppressing the deposition of sulfates by Ce addition made the Fe/beta catalyst a great SO2 tolerance. It was speculated that the outstanding performance of Ce doping Fe/beta catalysts made them attractive for practical application. (C) 2015 Elsevier B.V. All rights reserved.
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