期刊
ELECTROCHIMICA ACTA
卷 263, 期 -, 页码 47-52出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.electacta.2018.01.050
关键词
Water-in-ionic liquid electrolytes; Electrochemical stability windows; Aqueous rechargeable batteries
资金
- KIST Europe basic research funding
- German-Korean joint SME R&D project of ZIM-AIF
- German-Korean joint SME R&D project of MOTIE/KIAT
Several hydrophilic ionic liquids dissolved in water with different molalities are studied as water-in-ionic liquid supporting electrolytes. They exhibit wide electrochemical stability window from 3 to 4.4 V, high ionic conductivities and good flowability, making them promising supporting electrolytes for aqueous high-voltage rechargeable batteries. In such supporting electrolytes, enhanced redox activities of lithium insertion/ extraction in anodic TiO2 film at low negative potential and Fe3+/Fe2+ couple at moderate positive potential were observed. Cyclability of an aqueous TiO2/Fe2+ hybrid battery is demonstrated with a voltage of 1.7 V. (c) 2018 Elsevier Ltd. All rights reserved.
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