期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 24, 期 61, 页码 16209-16217出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201802706
关键词
C-H activation; cobalt; electrochemistry; electrosynthesis; heterocycles
资金
- DFG (Gottfried-Wilhelm-Leibniz award)
Carbon-heteroatom bonds represent omnipresent structural motifs of the vast majority of functionalized materials and bioactive compounds. C-H activation has emerged as arguably the most efficient strategy to construct C-Het bonds. Despite of major advances, these C-H transformations were largely dominated by precious transition metal catalysts, in combination with stoichiometric, toxic metal oxidants. Herein, we discuss the recent evolution of cobalt-catalyzed C-H activations that enable C-Het formations with electricity as the sole sustainable oxidant until May 2018.
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