期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 24, 期 33, 页码 8302-8305出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201801539
关键词
annulation; carbene catalysis; enantioselectivity; piperidones; pyrrolidones
资金
- Chinese Academy of Sciences
- National Natural Science Foundation of China [21425207, 21521002]
The N-heterocyclic carbene-catalyzed [2+3] and [2+4] annulations of alpha-chloroaldehydes with gamma-/delta-amino-alpha,beta-unsaturated ketones were developed, giving the corresponding pyrrolidones and piperidones in good yields with exclusive trans-selectivities and excellent enantioselectivities.
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