期刊
CHEMISTRY LETTERS
卷 47, 期 3, 页码 373-376出版社
CHEMICAL SOC JAPAN
DOI: 10.1246/cl.171093
关键词
Multielectron oxygen reduction; Particle-size effect; Kinetic model
资金
- MEXT KAKENHI [25107503]
- JSPS KAKENHI [16K1408606]
- Grants-in-Aid for Scientific Research [25107503, 16K14086] Funding Source: KAKEN
The light-intensity dependence (LID) of oxygen evolution using titanium(IV) oxide particles and electron acceptors under intense UV-LED irradiation was multimodal; in general, the LID changed from second to first order, and then fourth order in some cases. Such LID-order switching could reasonably be explained using a kinetic model in which the probability of multipleelectron (positive holes) accumulation in each particle governs the overall rates digitally.
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