4.4 Article

A Novel Nano-sized Catalyst CeO2-CuO/Hollow ZSM-5 for NO(x)( )Reduction with NH3

期刊

CHEMICAL RESEARCH IN CHINESE UNIVERSITIES
卷 34, 期 4, 页码 661-664

出版社

HIGHER EDUCATION PRESS
DOI: 10.1007/s40242-018-7333-9

关键词

Hollow-ZSM-5; Selective catalytic reduction; Hydrothermal method; NOx conversion

资金

  1. National Natural Science Foundation of China [21603213, 21677139]
  2. Fund of the Changchun Science and Technology Bureau, China [17DY004]
  3. Youth Innovation Promotion Association of Chinese Academy of Sciences [2018263]
  4. Development Program of the Science and Technology Department of Jilin Province, China [20180201088GX]

向作者/读者索取更多资源

Hollow-ZSM-5 was synthesized by a traditional hydrothermal method without alcohol, and a novel nano-sized Ce-Cu/hollow ZSM-5 sample was prepared by conventional incipient wetness impreganation. The catalysts were characterized by TEM, SEM, XRD, NMR and N-2 adsorption-desorption. The results indicate that the hollow-ZSM-5 has a good MFI structure with large surface area. The synthesized CeO2-CuO/hollow ZSM-5 showed an excellent catalytic activity for NO conversion(90% NOx conversion were obtained) in the temperature range of 340-550 degrees C under GHSV=480000 mL.g(-1) h(-1) due to its appropriate redox ability and acidity.

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