期刊
CHEMICAL RECORD
卷 18, 期 11, 页码 1531-1547出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/tcr.201800029
关键词
water oxidation catalyst; earth-abundant transition metal; polyoxometalate; metal oxide; metal complex
资金
- National Natural Science Foundation of China [21773096]
- Fundamental Research Funds for the Central Universities [lzujbky-2018-k0-8]
- Natural Science Foundation of Gansu [17JR5RA186]
Exploration of water oxidation catalyst (WOC) with excellent performance is the key for the overall water splitting reaction, which is a feasible strategy to convert solar energy to chemical energy. Although some compounds composed of noble metals, mainly Ru and Ir, have been reported to catalyze water oxidation with high efficiency, catalysts based on low-cost and earth-abundant transition metals are essential for realizing economical and large-scale light-driven water splitting. Various WOCs containing earth-abundant metals (mainly Mn, Fe, Co, Ni, Cu) have been utilized for visible light-driven water oxidation in recent years. In this Personal Account, we summarize our recent developments in WOCs based on earth-abundant transition metals including polyoxometalates (POMs), metal oxides or bimetal oxides, and metal complexes containing multidentate ligand scaffolds for visible light-driven water oxidation reaction.
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