期刊
CHEMICAL COMMUNICATIONS
卷 54, 期 67, 页码 9270-9273出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8cc02679c
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资金
- Japan Society for the Promotion of Science (JSPS) [26220911, 16K14478]
- MEXT
- JSPS [16J08114]
Photocatalytic H2O2 production via two-electron reduction of O-2 was realized by visible-light irradiation of a metal-organic framework, MIL-125-NH2, in the presence of TEOA and benzylalcohol. Deposition of NiO nanoparticles onto MIL-125-NH2 dramatically enhanced the catalytic activity. Further studies suggested that fast disproportionation of the O-2(center dot-) intermediate to H2O2 resulted in the enhancement.
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