期刊
CHEMICAL COMMUNICATIONS
卷 54, 期 51, 页码 6979-6982出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8cc03121e
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资金
- TALISMAN [TALI_C05-18]
- Deutscher Akademischer Austauschdienst (DAAD) [57314018]
Successful synthesis of the first transuranium metal-organic frameworks (TRU-MOFs) involving tetravalent Np4+ is reported. These compounds were obtained from the controlled hydrolysis of Np4+ in the presence of dicarboxylate ligands. The final structures contain the [Np6O4(OH)(4)(H2O)(6)](12+) unit, which were never crystallized before with tetravalent neptunium, associated with ditopic ligands.
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