4.7 Article

Facile fabrication of shape-controlled CoxMnyO beta nanocatalysts for benzene oxidation at low temperatures

期刊

CHEMICAL COMMUNICATIONS
卷 54, 期 17, 页码 2154-2157

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/c8cc00023a

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资金

  1. national key research and development program [2016YFC0203900, 2016YFC0203902]
  2. National Natural Science Foundation of China [21703037, 21773030]
  3. leading project of Fujian Province [2017H0049]

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We report a new strategy for the design and construction of CoxMnyO beta for C6H6 oxidation, a representative VOC. The nanostructures of CoxMnyO beta can be tuned from nanowires to needles, hollow/hierarchical microspheres and nanocubes. Moreover, different nanostructures of CoxMnyO beta show diverse textural/structural/surface properties, which in turn show strikingly different catalytic performances. Benefitting from its unique structural feature, nanocubic MnO2 exhibits a superior to considerably high activity for C6H6 oxidation at low temperatures.

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