期刊
CERAMICS INTERNATIONAL
卷 44, 期 14, 页码 17283-17289出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.ceramint.2018.06.189
关键词
P-type semiconducting gas sensor; NO2 sensing; SnO-SnO2 p-n heterojunction; Thin-film; RF-magnetron sputtering
资金
- MAT (Korea Institute for Advancement of Technology) - Korea Government (MOTIE: Ministry of Trade Industry and Energy) [N0001883]
- National Research Foundation of Korea (NRF) - Korea government (MSIP) [2017R1A2A2A14001213]
In this work, a high-performance p-type semiconducting gas sensor was successfully fabricated based on a SnO-SnO2 p-n heterojunction thin-film formed via a radio-frequency (RF)-magnetron sputtering process. The structure, morphology, and chemical composition of the deposited thin-film were investigated using scanning electron microscopy, X-ray diffraction, and X-ray photoelectron spectroscopy, indicating that the thin-film had a microcrystalline structure and a mixed SnO and SnO2 phase. Compared to the previously reported p-type metal oxide semiconductor-based gas sensors, the gas sensor in this study exhibited competitive sensing performance for NO2 gas with a maximum response of 4.35-10 ppm NO2 at a low operating temperature of 60 degrees C, although it was fabricated via a simple RF- magnetron sputtering process. Moreover, the SnO-SnO2 p-n heterojunction thin-film gas sensor exhibited a high sensing selectivity to NO2 gas. The enhanced NO2-sensing performance of the fabricated gas sensor at low operating temperatures is possibly attributed to the formation of the SnO-SnO2 p-n junctions at the surface of the thin-film. The importance of this work is in the successful fabrication of the high-performance p-type semiconducting gas sensor using a simple and conventional RF-magnetron sputtering process.
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