期刊
BIORESOURCE TECHNOLOGY
卷 264, 期 -, 页码 359-369出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.biortech.2018.06.013
关键词
Methane enrichment; Biogas upgrading; Methanation; Hydrogenation; In-situ; Ex-situ and Bioelectrochemical System
资金
- FutureGas project from Innovation Fund, Denmark - Innovationsfonden [5160-00006A]
Biogas upgrading technologies have received widespread attention recently and are researched extensively. Microbial biogas upgrading (biomethanation) relies on the microbial performance in enriched H-2 and CO2 environments. In this review, recent developments and applications of CH4 enrichment in microbial methanation processes are systematically reviewed. During biological methanation, either H-2 can be injected directly inside the anaerobic digester to enrich CH4 by a consortium of mixed microbial species or H-2 can be injected into a separate bioreactor, where CO2 contained in biogas is coupled with H-2 and converted to CH4, or a combination hereof. The available microbial technologies based on hydrogen-mediated CH4 enrichment, in particular ex-situ, in-situ and bioelectrochemical, are compared and discussed. Moreover, gas-liquid mass transfer limitations, and dynamics of bacteria-archaea interactions shift after H-2 injection are thoroughly discussed. Finally, the summary of existing demonstration, pilot plants and commercial CH4 enrichment plants based on microbial biomethanation are critically reviewed.
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