4.6 Article

Gapless quantum spin liquid ground state in the spin-1 antiferromagnet 6HB-Ba3NiSb2O9

期刊

PHYSICAL REVIEW B
卷 93, 期 21, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.93.214432

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资金

  1. French Agence Nationale de la Recherche under Grant SPINLIQ [ANR-12-BS04-0021]
  2. Universite Paris-Sud Grant MRM PMP
  3. Triangle de la physique [084004]
  4. National Sciences and Engineering Research Council (NSERC) of Canada

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We present an in-depth study of the magnetic properties of the spin-1 antiferromagnet 6HB-Ba3NiSb2O9. mu SR measurements demonstrate that this material shows no static magnetism down to temperatures as low as 20 mK, making it a likely candidate for a quantum spin liquid state. Sb-121 NMR shift measurements show that the local, intrinsic susceptibility levels off at temperatures below similar to 60 K. The NMR spin-lattice relaxation rate 1/T-1 is essentially constant in temperature and the muon relaxation rate exhibits a low-temperature relaxation plateau, all indications of gapless spin excitations. Our local probe measurements are discussed in the context of several theories proposed for this material.

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