期刊
ADVANCED FUNCTIONAL MATERIALS
卷 28, 期 32, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201802407
关键词
high-lying triplet; room-temperature phosphorescence; spin-orbital coupling; ternary emission; white light
类别
资金
- National Natural Science Foundation of China [51473063, 91233116, 51673083]
- National Key Basic Research and Development Program of China [2016YFB0401001, 2013CB834801, 2015CB655003]
- Postdoctoral Innovation Talent Support Project [BX201700097]
- China Postdoctoral Science Foundation [2017M620108]
Herein, a simple aza-aromatic compound dibenzo[a,c]phenazine (DPPZ), which exhibits single-molecule white light with a ternary emission, consisting of simultaneous fluorescence (S1S0) and dual room-temperature phosphorescence (RTP, T2S0 and T1S0) is reported. The Commission Internationale de l' Eclairage coordinates of DPPZ powder are (0.28, 0.33). To everyone's knowledge, this is the first case to achieve single-molecule white emission with ternary emission of fluorescence and dual RTP. This finding provides a prototype strategy to realize low-cost, stable pure organic single-molecule white light emission with three standard primary colors through further precise modulation of excited states.
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