期刊
ADVANCED FUNCTIONAL MATERIALS
卷 28, 期 8, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201705588
关键词
catalyst recovery; composites; metal-organic frameworks; nanoparticles; photocatalysis
类别
资金
- EPSRC IAA Partnership Development Award [RG/75759]
- Royal Society through a University Research Fellowship
- Ernest Oppenheimer Fund (Cambridge)
A new type of composite material involving the in situ immobilization of tin oxide nanoparticles (SnO2-NPs) within a monolithic metal-organic framework (MOF), the zeolitic imidazolate framework (ZIF)-8 is presented. SnO2@(mono)ZIF-8 exploits the mechanical properties, structural resilience, and high density of a monolithic MOF, while leveraging the photocatalytic action of the nanoparticles. The composite displays outstanding photocatalytic properties and represents a critical advance in the field of treating toxic effluents and is a vital validation for commercial application. Crucially, full retention of catalytic activity is observed after ten catalytic cycles.
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