期刊
ADVANCED FUNCTIONAL MATERIALS
卷 28, 期 13, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201707110
关键词
continuous-flow microreactors; core-shell metal-organic frameworks; covalent organic frameworks; metal-organic frameworks; photocatalysis
类别
资金
- National Research Foundation (NRF) of Korea - Korean government (MSIP) [NRF-2017R1A3B1023598]
- Ministry of Trade, Industry and Energy of Korea (MOTIE) [10052980]
Metal doped core-shell Metal-Organic Frameworks@Covalent Organic Frameworks (MOFs@COFs) are presented as a novel platform for photocatalysis. A palladium (Pd) doped MOFs@COFs in the form of Pd/TiATA@LZU1 shows excellent photocatalytic performance for tandem dehydrogenation and hydrogenation reactions in a continuous-flow microreactor and a batch system, indicating the great potential of the metal doped MOFs@COFs as a multifunctional platform for photocatalysis. Explanations for the performance enhancement are elucidated. An integrated dual-chamber microreactor coupled with the metal doped MOFs@COFs is introduced to demonstrate a concept of an intensified green photochemical process, which can be broadly extended to challenging liquid-gas tandem and cascade reactions.
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