期刊
ACS APPLIED MATERIALS & INTERFACES
卷 11, 期 3, 页码 2740-2744出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.8b03311
关键词
N-graphdiyne; nanosheets; interfacial synthesis; NADH; photocatalysis
资金
- National Natural Science Foundation of China [21604046]
- National Young Thousand Talents Program, Shandong Provincial Natural Science Foundation, China [ZR2016XJ004, ZR2018MB018]
Two-dimensional (2D) N-graphdiyne (N-GDY) nanosheets containing different number of N were synthesized by polymerization of triazine, pyrazine, and pyridine-based monomers at liquid/liquid interface. The configurations and nanostructures of N-GDY were well-characterized. The wettability changed to more hydrophilic as the N contents increased. The collected N-GDY was further employed as metal-free photocatalyst for NADH regeneration. The catalytic performance was related with the N content in the graphdiyne. The N3-GDY demonstrated the best activity. This strategy provided a new promising platform of designing unique 2D N-GDY with tunable performance in biorelated catalysis.
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