期刊
NATURE ENERGY
卷 2, 期 4, 页码 -出版社
NATURE PORTFOLIO
DOI: 10.1038/nenergy.2017.18
关键词
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资金
- US Department of Energy (DOE) SunShot Initiative under the Next Generation Photovoltaics 3 programme [DE-FOA-0000990]
- National Science Foundation [CITE-1230246, DMR-1534686]
- Ohio Research Scholar Program
- US Department of Energy SunShot Initiative under the Next Generation Photovoltaics 3 programme [DE-F0A-0000990, DE-AC36-08-G028308]
- Office of Science of the US Department of Energy [DE-AC02-05CH11231]
- National Natural Science Foundation of China (NSFC) [91422301]
- Division Of Materials Research
- Direct For Mathematical & Physical Scien [1230246] Funding Source: National Science Foundation
Tandem solar cells using only metal-halide perovskite sub-cells are an attractive choice for next-generation solar cells. However, the progress in developing efficient all-perovskite tandem solar cells has been hindered by the lack of high-performance low-bandgap perovskite solar cells. Here, we report efficient mixed tin-lead iodide low-bandgap (similar to 1.25 eV) perovskite solar cells with open-circuit voltages up to 0.85V and over 70% external quantum efficiencies in the infrared wavelength range of 700-900 nm, delivering a short-circuit current density of over 29 mAcm(-2) and demonstrating suitability for bottom-cell applications in all-perovskite tandem solar cells. Our low-bandgap perovskite solar cells achieve a maximum power conversion efficiency of 17.6% and a certified efficiency of 17.01% with a negligible current-voltage hysteresis. When mechanically stacked with a similar to 1.58 eV bandgap perovskite top cell, our best all-perovskite 4-terminal tandem solar cell shows a steady-state efficiency of 21.0%.
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