期刊
PHYSICAL REVIEW B
卷 94, 期 21, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.94.214105
关键词
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资金
- Ministry of Science and Technology of China [2016YFA0300504]
- National Science Foundation of China
- Strategic Priority Research Program (B) of the Chinese Academy of Sciences [XDB07020100]
- Fundamental Research Funds for the Central Universities
- Research Funds of Renmin University of China [10XNI038, 14XNLF06, 14XNLQ03, 14XNLQ07]
We comparably performed polarized Raman scattering studies of MoTe2 and WTe2. By rotating crystals to tune the angle between the principal axis of the crystals and the polarization of the incident/scattered light, we obtained the angle dependence of the intensities for all the observed modes, which is perfectly consistent with careful symmetry analysis. Combining these results with first-principles calculations, we clearly identified the observed phonon modes in the different phases of both crystals. Fifteen Raman-active phonon modes (10 A(g) + 5 B-g) in the high-symmetry phase 1T' -MoTe2 (300 K) were well assigned, and all the symmetry-allowed Raman modes (11 A(1) + 6 A(2)) in the low-symmetry phase T-d-MoTe2 (10 K) and 12 Raman phonons (8 A(1) + 4 A(2)) in T-d-WTe2 were observed and identified. The present paper provides basic information about the lattice dynamics in transition-metal dichalcogenides and may shed some light on the understanding of the extremely large magnetoresistance in this class of materials.
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