期刊
MATERIALS HORIZONS
卷 4, 期 5, 页码 915-923出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7mh00303j
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资金
- NSF [DMR 1420541]
- Cornell High Energy Synchrotron Source (CHESS)
- Princeton Center for Complex Materials
- NIH/NIGMS via NSF [DMR-1332208]
- National Science Foundation [DMR 1627428]
- Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy [DESC0008120]
- National Sciences and Engineering Council of Canada
Amorphous nanoparticles of the singlet fission chromophore 6,13-bis(triisopropylsilylethynyl) pentacene (TIPS-Pn) are fully crystallized through co-precipitation with a chemical additive. Time-resolved measurements indicate that singlet fission in the crystalline nanoparticles is quantitative, or lossless, whereas losses are evident in the amorphous nanoparticles as a result of frustrated triplet pair separation. Because triplet pairs formrapidly and separate slowly in amorphous material, mixed-phase samples are unable to compensate for these losses.
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