期刊
CHEMELECTROCHEM
卷 4, 期 11, 页码 2877-2883出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/celc.201700554
关键词
Doping; electrode materials; heteroatoms; microporosity; sodium ion batteries
资金
- Natural Science Foundation of China [21503071, 21501049]
- Fund of Key Scientific and Technological Project of Henan Province [172102210353, 162102210070]
The electronic environment and physicochemical property of carbon materials can be easily tailored and modulated by heteroatom doping. Herein, we demonstrate that net-like N, O, S triple-doped microporous carbon nanowires (NOS-MCNs) as an anode can be designed to improve the electrochemical performance of sodium ion batteries. Ammonium persulfate as oxidant can also provide a nitrogen and sulfur source for S-containing PPy. The N, O and S atoms are introduced into the carbon skeleton with activation and carbonization processes to modify the surface properties. As an anode, the material exhibits a high specific capacity and a long lifespan (approximate to 301 mAhg(-1) at 0.2 Ag-1 after 1000 cycles) as well as an excellent rate capability (158 mAhg(-1) at an extremely high current density of 10 Ag-1). This work offers a facile strategy to synthesize triple-doped porous carbon materials for sodium ion batteries and other energy-storage fields.
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