期刊
NANO ENERGY
卷 40, 期 -, 页码 233-239出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.nanoen.2017.08.022
关键词
Sodium dual-ion battery; Anion intercalation; Graphene-coated Na2Ti3O7; Coronene; Cycling life
类别
资金
- American Chemical Society Petroleum Research Fund [PRF 55708-DNI10]
- National Key Basic Research Program of China (973 Program) [2014CB239701]
- National Natural Science Foundation of China [51372116, 51504139, 51672128]
- Funding for Outstanding Doctoral Dissertation in NUAA [BCXJ16-07]
- Jiangsu Innovation Program for Graduate Education [KYLX16_0341]
- Priority Academic Program Development of Jiangsu Higher Education (PAPD)
- China Scholarship Council (CSC)
- U.S. Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office
- DOE Office of Science [DE-AC02-06CH11357]
Here we construct a novel sodium dual-ion battery (Na-DIB) with a conventional alkyl/alkylene carbonate electrolyte by using reduced-graphene-oxide-coated Na2Ti3O7 (NTO@G) as the anode and coronene, a polycyclic aromatic hydrocarbon (PAH), as the cathode. The coronene//NTO@G configuration delivers a specific energy of 77 W h kg(-1), based on the total active mass in both electrodes, and excellent cycling stability with 80% capacity retention after 5000 cycles. In addition, this device can work well in a wide range of temperatures from -20 to 40 degrees C. The results demonstrate a proof-of-concept Na-DIB that avoids the challenges of conventional dual-graphite DIBs by utilizing non-graphite intercalation anode and cathode, and a carbonate-based electrolyte without any additives.
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