期刊
NANO ENERGY
卷 36, 期 -, 页码 313-321出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.nanoen.2017.04.041
关键词
Inkjet printing; Silicon; Binder; Lithium-ion battery; PEDOT:PSS
类别
资金
- Natural Sciences and Engineering Research Council of Canada (NSERC)
- Canada Research Chair (CRC) Program
- Canada Foundation for Innovation (CFI)
- Ontario Research Fund (ORF)
- University of Western Ontario
- Province of Ontario
Herein we report the fabrication, optimization, and characterization of inkjet-printed thin film silicon anodes for lithium-ion batteries using commercial silicon nanoparticles. By comparing four different polymer binders, we demonstrate the critical role of binder on achieving good electrochemical performance of inkjet-printed silicon electrodes. Inkjet-printed silicon nanoparticle electrodes with conductive polymer PEDOT: PSS binder exhibit superior performance and durablity, with a capacity retention of over 1000 cycles at a depth-of-discharge of 1000 mA h g(-1). The working mechanism of the impact of the binders on inkjet-printed silicon electrodes is investigated and explained in detail via various characterization techniques, including scanning electron microscopy, Raman and infrared spectroscopy.
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