期刊
NANO ENERGY
卷 42, 期 -, 页码 69-89出版社
ELSEVIER
DOI: 10.1016/j.nanoen.2017.10.045
关键词
Hydrogen evolution; Hydrogen oxidation; Electrocatalysis; Non-precious metal; Nanomaterials
类别
资金
- National Natural Science Foundation of China [21603078]
- National Materials Genome Project [2016YFB0700600]
- National 1000 Young Talents Program of China
- University at Buffalo
- U.S. DOE EERE Fuel Cell Technologies Offices Incubator Program [DE-EE0006960]
- China Postdoctoral Science Foundation [2017M610470]
Hydrogen (H-2) is the most promising green energy resources to replace conventional fossil fuels due to the high mass energy density and renewability. The hydrogen evolution reaction (HER) and hydrogen oxidation reaction (HOR) are two reactions that play key roles in electrochemical energy storage and conversion with the sustainable H-2 as a medium. To date, the most efficient catalysts for production and conversion of hydrogen are based on noble metals. Therefore, the development of non-noble metal catalysts with high efficiency and low cost is of significant importance for the practical application of H-2 in different electrochemical energy technologies. In this review, we recapitulate the recent progress of developing non-noble metal-based electrocatalysts for HER and HOR and provide insights into the origins of catalytic performance enhancement. Fundamental understanding of the synthesis-structure-activity correlations, focusing on the HER/HOR mechanisms in acidic/alkaline media on studied non-noble metal catalysts are also discussed.
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