期刊
NANO ENERGY
卷 41, 期 -, 页码 681-686出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.nanoen.2017.10.026
关键词
Perovskite solar cells; Vacuum depositions; Hole transporting layers; Hole mobilities
类别
资金
- Ministry of Science and Technology of Taiwan [MOST 105-2112-M-007-016-MY3, MOST 105-2628-E-007-008-MY3]
- National Tsing Hua University
Hole transporting layers (HTLs) have critical roles in the performance of perovskite solar cells. In this study, films of the vacuum-deposited small molecule of Tris[4-(5-phenylthiophene-2-yl) phenyl] amine (TPTPA) are demonstrated as efficient HTL materials for perovskite solar cells. The horizontal molecular stacking of the TPTPA neat film leads to the exceptionally high hole drift mobility of 7 x 10(-3) cm(2) V-1 s(-1), among the highest values observed in the organic molecular neat films. By doping with MoO3, a clear charge transfer state is formed and the hole mobility further increases to 3.6 x 10(-2) cm(2) V-1 s(-1). Both normal-and inverted-structured perovskite solar cells utilizing these HTLs are prepared and optimized; they show high power conversion efficiencies of 17-18%.
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