期刊
APPLIED SURFACE SCIENCE
卷 392, 期 -, 页码 991-1003出版社
ELSEVIER
DOI: 10.1016/j.apsusc.2016.09.150
关键词
Laser ablation synthesis in liquid; Composites; Core-shell; Polymerization; Grafting; Encapsulation; Dispersion
类别
资金
- Mercator Research Center Ruhr [An-2015-0065]
Nanoparticle synthesis by laser ablation in liquids has attracted attention from researchers worldwide the past few years and the integration of these nanoparticles in functional materials such as nanoparticle-polymer composites, represents a natural next step. Such nanointegration into polymers can be achieved by the ex situ dispersion of laser-synthesized inorganic nanoparticles in polymer matrices and the in situ encapsulation/grafting of nanoparticles with polymers/monomers during synthesis. Because the nanoparticle shell and the polymer matrix may be identical, this method often does not require the use of dispersants or matrix binders and constitutes a new avenue for direct particle-polymer coupling. In this perspective review, we summarize the methodologies for in situ and ex situ laser prototyping of nanoparticle-polymer composites (LaNPC) and downstream bulk-processing techniques. The determinants of polymer-solvent-laser parametrization for aimed physical and chemical properties of the composites are discussed. By highlighting representative works related to a variety of promising applications, the advantageous features of this technique are demonstrated. Finally, the challenges and prospects of LaNPC are outlined and a perspective is given regarding how the recent research findings reviewed changed the research direction in the field. (C) 2016 Elsevier B.V. All rights reserved.
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