期刊
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
卷 513, 期 -, 页码 117-124出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.colsurfa.2016.11.040
关键词
g-C3N4/Ag/BiVO4; Heterostructure; Photocatalysis; Visible light
资金
- National Natural Science Fundation of China [21407059, 21576112, 51404108, 61308095]
- Science and Technology Research Project of the Department of Education of Jilin Province [2015220]
- Science Development Project of Jiangsu Province [BK20140527]
The ternary heterostructured g-C3N4/Ag/BiVO4 photocatalyst was successfully fabricated by a facile in situ precipitation method. The as-prepared g-C3N4/Ag/BiVO4 heterostructures included g-C3N4 and Ag nanoparticles (NPs) assembling on the surface of leaf-like BiVO4 nanostructures. The g-C3N4/Ag/BiVO4 composite exhibited higher photocatalytic activity than pure g-C3N4, BiVO4, Ag/BiVO4 and g-C3N4/BiVO4. The enhanced photocatalytic performance could be attributed to an efficient separation of electron-hole pairs through a ternary composite system, in which Ag nanoparticles acted as electron sinks. In addition, the quenching effects of different scavengers showed that the reactive O-2(center dot-) and (OH)-O-center dot play the major role in the Rh B decolorization. (C) 2016 Elsevier B.V. All rights reserved.
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